Superconductivity and strong interactions in a tunable moiré quasicrystal.

Electronic states in quasicrystals generally preclude a Bloch description1, rendering them fascinating and enigmatic. Owing to their complexity and scarcity, quasicrystals are underexplored relative to periodic and amorphous structures. Here we introduce a new type of highly tunable quasicrystal easily assembled from periodic components. By twisting three layers of graphene with two different twist angles, we form two mutually incommensurate moiré patterns. In contrast to many common atomic-scale quasicrystals2,3, the quasiperiodicity in our system is defined on moiré length scales of several nanometres. This 'moiré quasicrystal' allows us to tune the chemical potential and thus the electronic system between a periodic-like regime at low energies and a strongly quasiperiodic regime at higher energies, the latter hosting a large density of weakly dispersing states. Notably, in the quasiperiodic regime, we observe superconductivity near a flavour-symmetry-breaking phase transition4,5, the latter indicative of the important role that electronic interactions play in that regime. The prevalence of interacting phenomena in future systems with in situ tunability is not only useful for the study of quasiperiodic systems but may also provide insights into electronic ordering in related periodic moiré crystals6-12. We anticipate that extending this platform to engineer quasicrystals by varying the number of layers and twist angles, and by using different two-dimensional components, will lead to a new family of quantum materials to investigate the properties of strongly interacting quasicrystals.

Multiple-scale structures: from Faraday waves to soft-matter quasicrystals.

For many years, quasicrystals were observed only as solid-state metallic alloys, yet current research is now actively exploring their formation in a variety of soft materials, including systems of macromolecules, nanoparticles and colloids. Much effort is being invested in understanding the thermodynamic properties of these soft-matter quasicrystals in order to predict and possibly control the structures that form, and hopefully to shed light on the broader yet unresolved general questions of quasicrystal formation and stability. Moreover, the ability to control the self-assembly of soft quasicrystals may contribute to the development of novel photonics or other applications based on self-assembled metamaterials. Here a path is followed, leading to quantitative stability predictions, that starts with a model developed two decades ago to treat the formation of multiple-scale quasiperiodic Faraday waves (standing wave patterns in vibrating fluid surfaces) and which was later mapped onto systems of soft particles, interacting via multiple-scale pair potentials. The article reviews, and substantially expands, the quantitative predictions of these models, while correcting a few discrepancies in earlier calculations, and presents new analytical methods for treating the models. In so doing, a number of new stable quasicrystalline structures are found with octagonal, octadecagonal and higher-order symmetries, some of which may, it is hoped, be observed in future experiments.

Controlled self-assembly of periodic and aperiodic cluster crystals.

Soft particles are known to overlap and form stable clusters that self-assemble into periodic crystalline phases with density-independent lattice constants. We use molecular dynamics simulations in two dimensions to demonstrate that, through a judicious design of an isotropic pair potential, one can control the ordering of the clusters and generate a variety of phases, including decagonal and dodecagonal quasicrystals. Our results confirm analytical predictions based on a mean-field approximation, providing insight into the stabilization of quasicrystals in soft macromolecular systems, and suggesting a practical approach for their controlled self-assembly in laboratory realizations using synthesized soft-matter particles.

Comment on "quantum quasicrystals of spin-orbit-coupled dipolar bosons".

A Comment on the Letter by S. Gopalakrishnan, I. Martin, and E. A. Demler, Phys. Rev. Lett. 111, 185304 (2013).. The authors of the Letter offer a Reply.

Surpassing fundamental limits of oscillators using nonlinear resonators.

In its most basic form an oscillator consists of a resonator driven on resonance, through feedback, to create a periodic signal sustained by a static energy source. The generation of a stable frequency, the basic function of oscillators, is typically achieved by increasing the amplitude of motion of the resonator while remaining within its linear, harmonic regime. Contrary to this conventional paradigm, in this Letter we show that by operating the oscillator at special points in the resonator's anharmonic regime we can overcome fundamental limitations of oscillator performance due to thermodynamic noise as well as practical limitations due to noise from the sustaining circuit. We develop a comprehensive model that accounts for the major contributions to the phase noise of the nonlinear oscillator. Using a nanoelectromechanical system based oscillator, we experimentally verify the existence of a special region in the operational parameter space that enables suppressing the most significant contributions to the oscillator's phase noise, as predicted by our model.

Optimal operating points of oscillators using nonlinear resonators.

We demonstrate an analytical method for calculating the phase sensitivity of a class of oscillators whose phase does not affect the time evolution of the other dynamic variables. We show that such oscillators possess the possibility for complete phase noise elimination. We apply the method to a feedback oscillator which employs a high Q weakly nonlinear resonator and provide explicit parameter values for which the feedback phase noise is completely eliminated and others for which there is no amplitude-phase noise conversion. We then establish an operational mode of the oscillator which optimizes its performance by diminishing the feedback noise in both quadratures, thermal noise, and quality factor fluctuations. We also study the spectrum of the oscillator and provide specific results for the case of 1/f noise sources.

Passive phase noise cancellation scheme.

We introduce a new method for reducing phase noise in oscillators, thereby improving their frequency precision. The noise reduction is realized by a passive device consisting of a pair of coupled nonlinear resonating elements that are driven parametrically by the output of a conventional oscillator at a frequency close to the sum of the linear mode frequencies. Above the threshold for parametric instability, the coupled resonators exhibit self-oscillations which arise as a response to the parametric driving, rather than by application of active feedback. We find operating points of the device for which this periodic signal is immune to frequency noise in the driving oscillator, providing a way to clean its phase noise. We present results for the effect of thermal noise to advance a broader understanding of the overall noise sensitivity and the fundamental operating limits.

Homoclinic orbits and chaos in a pair of parametrically driven coupled nonlinear resonators.

We study the dynamics of a pair of parametrically driven coupled nonlinear mechanical resonators of the kind that is typically encountered in applications involving microelectromechanical systems (MEMS) and nanoelectromechanical systems (NEMS). We take advantage of the weak damping that characterizes these systems to perform a multiple-scales analysis and obtain amplitude equations, describing the slow dynamics of the system. This picture allows us to expose the existence of homoclinic orbits in the dynamics of the integrable part of the slow equations of motion. Using a version of the high-dimensional Melnikov approach, developed by G. Kovacic and S. Wiggins [Physica D 57, 185 (1992)], we are able to obtain explicit parameter values for which these orbits persist in the full system, consisting of both Hamiltonian and non-Hamiltonian perturbations, to form so-called Silnikov orbits, indicating a loss of integrability and the existence of chaos. Our analytical calculations of Silnikov orbits are confirmed numerically.

Signal amplification by sensitive control of bifurcation topology.

We describe a novel amplification scheme based on inducing dynamical changes to the topology of a bifurcation diagram of a simple nonlinear dynamical system. We have implemented a first bifurcation-topology amplifier using a coupled pair of parametrically driven high-frequency nanoelectromechanical systems resonators, demonstrating robust small-signal amplification. The principles that underlie bifurcation-topology amplification are simple and generic, suggesting its applicability to a wide variety of physical, chemical, and biological systems.

Intrinsic localized modes in parametrically driven arrays of nonlinear resonators.

We study intrinsic localized modes (ILMs), or solitons, in arrays of parametrically driven nonlinear resonators with application to microelectromechanical and nanoelectromechanical systems (MEMS and NEMS). The analysis is performed using an amplitude equation in the form of a nonlinear Schrödinger equation with a term corresponding to nonlinear damping (also known as a forced complex Ginzburg-Landau equation), which is derived directly from the underlying equations of motion of the coupled resonators, using the method of multiple scales. We investigate the creation, stability, and interaction of ILMs, show that they can form bound states, and that under certain conditions one ILM can split into two. Our findings are confirmed by simulations of the underlying equations of motion of the resonators, suggesting possible experimental tests of the theory.

Pattern selection in parametrically driven arrays of nonlinear resonators.

We study the problem of pattern selection in an array of parametrically driven nonlinear resonators with application to microelectromechanical and nanoelectromechanical systems, using an amplitude equation recently derived by Bromberg, Cross, and Lifshitz [Phys. Rev. E 73, 016214 (2006)]. We describe the transitions between standing-wave patterns of different wave numbers as the drive amplitude is varied either quasistatically, abruptly, or as a linear ramp in time. We find interesting hysteretic effects, which are confirmed by numerical integration of the original equations of motion of the interacting nonlinear resonators.

Signatures for a classical to quantum transition of a driven nonlinear nanomechanical resonator.

We seek the first indications that a nanoelectromechanical system (NEMS) is entering the quantum domain as its mass and temperature are decreased. We find them by studying the transition from classical to quantum behavior of a driven nonlinear Duffing resonator. Numerical solutions of the equations of motion, operating in the bistable regime of the resonator, demonstrate that the quantum Wigner function gradually deviates from the corresponding classical phase-space probability density. These clear differences that develop due to nonlinearity can serve as experimental signatures, in the near future, that NEMS resonators are entering the quantum domain.

Phason dynamics in nonlinear photonic quasicrystals.

We study the dynamics of phasons in a nonlinear photonic quasicrystal. The photonic quasicrystal is formed by optical induction, and its dynamics is initiated by allowing the light waves inducing the quasicrystal to nonlinearly interact with one another. We show quantitatively that, when phason strain is introduced in a controlled manner, it relaxes through the nonlinear interactions within the photonic quasicrystal. We establish experimentally that the relaxation rate of phason strain in the quasicrystal is substantially lower than the relaxation rate of phonon strain, as predicted for atomic quasicrystals. Finally, we monitor and identify individual 'atomic-scale' phason flips occurring in the photonic quasicrystal as its phason strain relaxes, as well as noise-induced phason fluctuations.

Wave and defect dynamics in nonlinear photonic quasicrystals.

Quasicrystals are unique structures with long-range order but no periodicity. Their properties have intrigued scientists ever since their discovery and initial theoretical analysis. The lack of periodicity excludes the possibility of describing quasicrystal structures with well-established analytical tools, including common notions like Brillouin zones and Bloch's theorem. New and unique features such as fractal-like band structures and 'phason' degrees of freedom are introduced. In general, it is very difficult to directly observe the evolution of electronic waves in solid-state atomic quasicrystals, or the dynamics of the structure itself. Here we use optical induction to create two-dimensional photonic quasicrystals, whose macroscopic nature allows us to explore wave transport phenomena. We demonstrate that light launched at different quasicrystal sites travels through the lattice in a way equivalent to quantum tunnelling of electrons in a quasiperiodic potential. At high intensity, lattice solitons are formed. Finally, we directly observe dislocation dynamics when crystal sites are allowed to interact with each other. Our experimental results apply not only to photonics, but also to other quasiperiodic systems such as matter waves in quasiperiodic traps, generic pattern-forming systems as in parametrically excited surface waves, liquid quasicrystals, and the more familiar atomic quasicrystals.

Synchronization by reactive coupling and nonlinear frequency pulling.

We present a detailed analysis of a model for the synchronization of nonlinear oscillators due to reactive coupling and nonlinear frequency pulling. We study the model for the mean field case of all-to-all coupling, deriving results for the initial onset of synchronization as the coupling or nonlinearity increase, and conditions for the existence of the completely synchronized state when all the oscillators evolve with the same frequency. Explicit results are derived for the Lorentzian, triangular, and top-hat distributions of oscillator frequencies. Numerical simulations are used to construct complete phase diagrams for these distributions.

Response of discrete nonlinear systems with many degrees of freedom.

We study the response of a large array of coupled nonlinear oscillators to parametric excitation, motivated by the growing interest in the nonlinear dynamics of microelectromechanical and nanoelectromechanical systems (MEMS and NEMS). Using a multiscale analysis, we derive an amplitude equation that captures the slow dynamics of the coupled oscillators just above the onset of parametric oscillations. The amplitude equation that we derive here from first principles exhibits a wave-number dependent bifurcation similar in character to the behavior known to exist in fluids undergoing the Faraday wave instability. We confirm this behavior numerically and make suggestions for testing it experimentally with MEMS and NEMS resonators.

Photonic quasicrystals for nonlinear optical frequency conversion.

We present a general method for the design of 2-dimensional nonlinear photonic quasicrystals that can be utilized for the simultaneous phase matching of arbitrary optical frequency-conversion processes. The proposed scheme--based on the generalized dual-grid method that is used for constructing tiling models of quasicrystals--gives complete design flexibility, removing any constraints imposed by previous approaches. As an example we demonstrate the design of a color fan--a nonlinear photonic quasicrystal whose input is a single wave at frequency omega and whose output consists of the second, third, and fourth harmonics of omega, each in a different spatial direction.

Synchronization by nonlinear frequency pulling.

We analyze a model for the synchronization of nonlinear oscillators due to reactive coupling and nonlinear frequency pulling motivated by the physics of arrays of nanoscale oscillators. We study the model for the mean field case of all-to-all coupling, deriving results for the onset of synchronization as the coupling or nonlinearity increase, and the fully locked state when all the oscillators evolve with the same frequency.

Symmetry of magnetically ordered three-dimensional octagonal quasicrystals.

The theory of magnetic symmetry in quasicrystals, described in a companion paper [Lifshitz & Even-Dar Mandel (2004). Acta Cryst. A60, 167-178], is used to enumerate all three-dimensional octagonal spin point groups and spin-space-group types and calculate the resulting selection rules for neutron diffraction experiments.